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Assessing the role of static lengthscales behind glassy dynamics in polydisperse hard disks

机译:评估静态长度尺度在玻璃体动力学中的作用   多分散硬盘

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摘要

The possible role of growing static order in the dynamical slowing downtowards the glass transition has recently attracted considerable attention. Onthe basis of random first-order transition (RFOT) theory, a new method tomeasure the static correlation length of amorphous order, called "point-to-set(PTS)" length, has been proposed, and used to show that the dynamic lengthgrows much faster than the static length. Here we study the nature of the PTSlength, using a polydisperse hard disk system, which is a model that is knownto exhibit a growing hexatic order upon densification. We show that the PTScorrelation length is decoupled from the steeper increase of the correlationlength of hexatic order, while closely mirroring the decay length of two-bodydensity correlations. Our results thus provide a clear example that other formsof order can play an important role in the slowing down of the dynamics,casting a serious doubt on the order agnostic nature of the PTS length and itsrelevance to slow dynamics, provided that a polydisperse hard disk system is atypical glass former.
机译:最近,逐渐增加的静态阶跃在向玻璃过渡的动力学减慢中可能发挥的作用引起了人们的极大关注。基于随机一阶跃迁(RFOT)理论,提出了一种测量非晶态静态相关长度的新方法,称为“点对集(PTS)”长度,用于表明动态长度的增长。比静态长度快得多。在这里,我们使用多分散硬盘系统研究了PTS长度的性质,该系统是一种已知在致密化后具有不断增长的六价序的模型。我们显示,PTS相关长度与六阶相关长度的急剧增加解耦,同时紧密反映了两体相关的衰减长度。因此,我们的结果提供了一个清晰的例子,即其他形式的有序形式在减慢动力学过程中可能起重要作用,如果多分散硬盘系统对PTS长度的顺序不可知性及其与慢速动力学的相关性提出了严重怀疑。是非典型的玻璃成型机。

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    Russo, John; Tanaka, Hajime;

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  • 年度 2015
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